I gotta say that Bloodfang Armor (Rogue T2) is the best Item set. Classic Rogue look from Vanilla!
All of the tier Six's were perfect for each class, but I'd have to go Paladin tier 6, hands down.. It perfectly represented the class. The armor reflected every spec as a "I'm going to cause some divine retribution" type of class.
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If I have to chose between two gear sets it would be between the Tier 1 and Tier 2 Warrior sets. Vanilla with it's epic 40-man raid when it was actually possible to find 40 people that would sign every night. The winnner of the two would be Tier 2 because my warrior who is still parked at Level 70 and only got to see one Karazhan run still has the Tier 2 boots. Ah the good old days :)
Hunter dungeon set 1, since it's the only one I ever got a significant amount of pieces for.
The T1 set. It was the first time for tier gear and it just really felt epic,
Warrior Wrath set, and I mean the stuff from Molten Core. I mean, the headpiece looks like you ripped SAW's reverse bear trap right offa your head and gave him the finger (which is probably why it gives +15 strength). In addition to that, the shoulders look perfect for charging people with YOUR HEAD, and you've got tusks on your DESTROYED BEAR-TRAP HELMET so you can PUMMEL those MISERABLE FOES like a real MAN or woMAN. The rest of the set looks like it was made OF BONE so would be perfect for PUMMELING MORE with your BONE ARMORED HANDS. Combine with a draconian deflector and Doom's Edge, and you've got some ownage right thar :3I out.
I love warlock tier 8, mostly just because of how deliciously evil it looks.
I liked the Balance druid tier 10 because it was the first set I ever completed, big sense of accomplishment there, hehe.
I still think all the tier 2 sets were the best and the most colorful haha but as always i give my 1st place to the tier 2 paladin just because of its cool design
Giantstalkers because the shoulder's and helmet made me look like a Mecha Orc!
I'd have to go with the priest tier 10. I dunno why but I always loved the color scheme of it. Also, the 4 piece bonus was pretty great too =)
Hands Down the Best Tier Set has got to be Cataclysm Harness! I mean who doesn't want to walk around with Molten Rock on your armor, and if Paired with Claw of Molten Fury and Fist of Molten Fury it just made the Whole suit come together in one Kick Butt package!