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I think I'd have to go with the Healing Priest T10 set, mostly because it was the first set I ever completed. That and I love the shoulders.
i would have to say the rogue t10 because if you ever saw the movie 9 it looks like a spitting image almost of the rag doll charactersand the fact that most druids were stealing the knock off pieces from ICC made it a versatile and sweet looking Tier
Shaman heroic t10. Matched perfectly to Northrend.
i really love the tier 2 priest set, will always be my favorite because of how detailed it looks and the set bonus was a plus heh that plus equipping my benediction/anathema is very nostalgic, been playing my priest for 6 years and going now and i have every set in my bank=)
I liked the T10 gear, mainly because it was the first time I ever had any tier gear. I had never been in a raiding guild that got into raiding enough to get any gear.
My T1 Cenarion Raiment, for my Druid, is the only Tier I have not deleted. I still break it out once in a while to remember the good times when this game was about larger guilds and heaps of patience. Made acquiring the full 8 piece set more rewarding.
I myself absolutely loved the Warrior Dreadnaught's set. When I laid eyes on it, it just looked so amazing with all the skulls and light blue particles. I still wish I could have gotten the full set.Dreadnaught's Battlegear
I am gonna have to go with Shaman T-1 Earthfury. Tis was my first tier set when I started playing and the graphics on it are just beautiful. One of my happiest moments was when the boots drop and I have won them. First epic I ever got.Droopox
My favourite was Warlock Tier 4. As I am playing Undead Lock for early start of WoW till present days this set looks awesome on him, like one of my favourite demon: Voidwalker. And this some kind of void or vortex effect around helm was pretty nice, showing true potencial of Lock.
I think it's Dk's T10, cause you just look like a scourge general and it's so cool!
I kinda gotta say there was nothing more awesome than Bloodfang Leather. That or the Pally Power Ranger gear. Also, I'm kinda partial to the new hunter "murloc" tier and the mage T-11 :)